Synthesis and Extraction Performance of 5-decylsalicylaldoxime Copper Extractant
           
View Full Text  View/Add Comment  Download reader
DOI:DOI:10.3969/j.issn.1007-7545.2011.07.002
KeyWord:metallurgical technology; copper extraction; synthesis; 5-decylsalicylaldoxime
                 
AuthorInstitution
ZHAO Shuang-hui 1.湘潭大学 化学学院,湖南湘潭 ;2.清华大学 化学系生命有机磷化学及化学生物学教育部重点实验室 北京
LUO Jun-qi 1.湘潭大学 化学学院,湖南湘潭 ;2.清华大学 化学系生命有机磷化学及化学生物学教育部重点实验室 北京
CHENG Chang-mei 清华大学 化学系生命有机磷化学及化学生物学教育部重点实验室 北京
CHEN Lang-qiu 湘潭大学 化学学院,湖南湘潭
LI Lin-yan 清华大学 核能与新能源技术研究院,北京
XU Sheng-ming 清华大学 核能与新能源技术研究院,北京
Hits: 2802
Download times: 31
Abstract:
      A novel copper extractant 5-decylsalicylaldoxime is synthesized with the use of a cheap mixture by-product, 5-decylsalicylaldoxime, from the petrochemical industry. The optimal condition is, n(decylphenol):n(magnesium):n(paraformaldehyde)=1:0.65:2.8, reaction time 5h for the formylation reaction and n(decylphenol):n(hydroxylamine hydrochloride)=1:1, reaction time 1h for the oximation reaction. Under this condition, the yield of the desired product reaches to 75.9% (based on decylphenol) with 99.0% purity (determined by GC). The structure is elucidated by MS, NMR and EA analysis. It is indicated by the comparison with the M5640 and M5774 that the extraction performance of the product is of high copper load capability (6.36 g/L), good copper selectivity over iron (β[Cu/Fe]?=1340), the extracting and stripping balance time are short, the extracting rate is more than 98% and the stripping extracting rate is more than90% through only one stage.
Close