Electrokinetic and Chemical Eluviation Combined Remediation of Uranium Contaminated Soil
Received:April 20, 2024   Revised:June 02, 2024   Accepted:June 03, 2024      Published Online:November 17, 2024
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DOI:doi:10.3969/j.issn.1007-7545.2024.12.013
KeyWord:uranium soil pollution; chemical leaching; electrokinetic and chemical eluviation combined remediation
                    
AuthorInstitution
JIANG Fangrong 东华理工大学
PAN Jinli 宁夏回族自治区核地质调查院(宁夏回族自治区放射性地质研究所)
JIANG Wenbo 东华理工大学
SONG Yong 江西省地质局有色地质大队
GAO Bai 东华理工大学
MA Wenjie 东华理工大学
ZHAO Chongzhen 东华理工大学
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Abstract:
      The problem of radioactive contamination of the soil around the mine poses a threat to the ecological environment and human health, and it is urgent to study the efficient remediation technology of uranium contaminated soil. Taking the radioactive contaminated soil in a uranium mining area as the research object to explore the optimal process parameters for uranium removal with different leaching solvent types, leaching solvent concentrations, liquid-solid ratio and compound leaching solvent ratio. The results show that there are significant differences in the removal performance of uranium from uranium contaminated soil by chemical leaching solvents, which is inorganic acid (48.70%) > organic acid (31.91%)> chelating agent (23.31%) > inorganic salts (17.26%). The combined use of composite leaching solvent and electrochemical leaching method can effectively improve the removal rate of uranium in contaminated soil, in which the average removal rate of uranium in contaminated soil is 59.75%, which is 13.37 percentage points higher than that of single chemical leaching under the optimal parameters of voltage of 30 V, composite concentration of citric acid + ferric chloride of 0.1 mol/L+7.5 g/L, liquid-solid ratio of 5 mL/g and temperature of 25 ℃.
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